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Beilstein J. Org. Chem. 2011, 7, 82–93, doi:10.3762/bjoc.7.12
Graphical Abstract
Scheme 1: Alkyne metathesis based on the Katz mechanism.
Scheme 2: Reaction patterns of alkyne metathesis.
Scheme 3: Typical examples from traditional catalyst systems.
Scheme 4: Ligand synthesis and catalyst design.
Scheme 5: Catalysts synthesis using high- and low-oxidation-state routes (for 6a, X = Li or K; for 6b, X = K)....
Figure 1: Alkylidyne complexes 9 and 10.
Scheme 6: Design strategy of Fürstner’s new system.
Scheme 7: Synthetic routes of Fürstner’s new catalysts.
Scheme 8: Lewis acid addition of 26 and 28.
Scheme 9: Preparation of the silanolate–alkylidyne tungsten complex 39.